- 作者: Chen Yang, Feng Shuang and Yi Jing Yan
- 中文摘要: We present a method of implementing the generalized Redfield theory on the calculation of femtosecond transient absorption spectrum of molecular systems in condensed phases. Numerical demonstration is carried out in a model Brownian molecular system involving two Morse potential surfaces. Intramolecular vibrational relaxation, its relation to the spectral density, its spectroscopic signature, and the temperature effect are analyzed.
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